Transiently stimulated second-harmonic generation from silicon nanogratings

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Authors

An, Yong Q.
Diebold, Alain C.

Issue Date

2017-11-29

Type

Article

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Keywords

nanotechnology , silicon nanogratings , second-harmonic (SH) light , nanoscale measurement , transiently stimulated SHG , high-harmonic generation , nonlinear optics , photonics

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Alternative Title

Physical Review B

Abstract

We observe that second-harmonic (SH) light generated by a femtosecond probe pulse from Si nanograting surfaces can be enhanced by a correlating pump pulse. Time-resolved anisotropy analysis shows that the enhancement arises from transient stimulation by the pump because it polarizes the periodically distributed charge from the probe photoinjection. In addition, dipole and quadrupole SH components are stimulated differently depending on the pump polarization. This effect reveals ultrafast SH dynamics in centrosymmetric materials and provides guidance for measuring nanoscale features.

Description

Citation

An, Y. Q., & Diebold, A. C. (2017). Transiently stimulated second-harmonic generation from silicon nanogratings. Physical Review B, 96(20), 201306. doi:10.1103/PhysRevB.96.201306

Publisher

American Physical Society

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PubMed ID

DOI

ISSN

2469-9950

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